Design of Heterogeneous Catalysts

This long-awaited reference source is the first book to focus on this important and hot topic. As such, it provides examples from a wide array of fields where catalyst design has been based on new insights and understanding, presenting such modern and important topics as self-assembly, nature-inspired catalysis, nano-scale architecture of surfaces and theoretical methods. With its inclusion of all the useful and powerful tools for the rational design of catalysts, this is a true "must have" book for every researcher in the field.

Autorentext
Umit S. Ozkan is a Professor of Chemical Engineering at the Ohio State University. Her research interests include heterogeneous catalysis and its applications to energy and environmental protection. She has edited five books, written over 150 refereed publications and has five patents. She served as the Co-chair of the Continuing Symposia in Catalysis for the Colloids and Surface Chemistry Division (1994-2000), Secretary of the Petroleum Chemistry Division (1998-99), and as President of the Petroleum Chemistry Division (2002-03) of the ACS. She is currently the Secretary of the North American Catalysis Society and a Director of the Catalysis and Reaction Engineering Division of the American Institute of Chemical Engineers. Professor Ozkan is also on the Editorial Board of Journal of Molecular Catalysis, Catalysis Letters, Topics in Catalysis, The Royal Society of Chemistry Catalysis Book Series and Catalysis Today.

Klappentext
Heterogeneous catalysts provide a surface for a chemical reaction to take place on, as it is in a different phase to the reactants. This reference book brings together examples from a wide array of fields where catalyst design has been based on new insights and understanding. Modern and important topics such as self-assembly, nature-inspired catalysis, nano-scale architecture of surfaces and theoretical methods are addressed. With its inclusion of all the useful and powerful tools for the rational design of catalysts, this is a true "must have" book every researcher in the field. From the Contents: * Use of Oxide Nanoligands in Designing/Controlling Actives Sites * Optimal Design of Hierarchically Structured Porous Catalysts * Use of Dendrimers in Catalytic Design * Rational Design Strategies for Industrial Catalysts * Chiral Modification of Catalytic Surfaces * Catalytic Nanomotors * Rational Design and High-Throughput Screening of Metal Open Frameworks for Gas Separation and Catalysis * Design of Bimetallic Hydrogenation Catalysts: From Model Surfaces to Supported Catalysts * Self-Assembled Materials for Catalysis * Theory-Aided Catalyst Design * Use of In-Situ XAS Techniques for Catalysts' Characterization and Design * Catalyst Design Through Dual Templating

Inhalt
USE OF OXIDE LIGANDS IN DESIGNING CATALYTIC ACTIVE SITES Introduction Molecular Structural Determination of Supported Metal Oxide Catalysts with In Situ Raman Spectroscopy Characterization of AlOx, TiOx, and ZrOx Surface-Modified SiO2 Anchoring Site of Surface M1Ox species on Supported M2Ox/SiO2 Molecular Structure of Dehydrated Supported V2O5/SiO2 and V2O5/M2Ox/SiO2 Catalyst Systems Molecular Structure of Dehydrated Supported M0O3/SiO2 and M0O3/M2Ox/SiO2 Catalyst Systems Molecular Structure of Dehydrated Supported Re2O7/SiO2 and Re2O7/M2Ox/SiO2 Catalyst Systems Electronic Structure of Dehydrated Supported MOx/SiO2 and M1Ox/M2Ox/SiO2 Catalysts via In Situ UV-Vis Spectroscopy Determination of Surface Kinetic Parameters Redox Surface Reactivity of Model Supported M1Ox/SiO2 Catalysts Redox Surface Reactivity of Supported M1Ox/M2Ox/SiO2 Catalysts OPTIMAL DESIGN OF HIERARCHICALLY STRUCTURED POROUS CATALYSTS Introduction Optimizing Mesopore Connectivity and Shape Optimizing Catalysts by Macroscopic Distributions in Activity Optimal Design of the Highway Network USE OF DENDRIMERS IN CATALYST DESIGN Introduction Modified Dendrimer Catalysts Indirect Effects of Dendrimer Architecture Catalysis by Dendrimer Encapsulated Nanoparticles Dendrimer Templated Nanocages RATIONAL DESIGN STRATEGIES FOR INDUSTRIAL CATALYSTS Introduction The First Stages Toward Commercialization of a Catalyst Catalyst Discovery to Commercialization Example 1: Automobile Pollution Abatement Catalyst System Example 2: Dehydrogenation of Light Alkanes Example 3: Petroleum Refining - Fluid Catalytic Cracking CHIRAL MODIFICATION OF CATALYTIC SURFACES Introduction Modification of Metal Surfaces by Cinchona Alkaloid and Related Compounds Modification of Metal Surfaces by Tartaric Acid and Related Compounds CATALYTIC NANOMOTORS Introduction The Propulsion Mechanism of Catalytic Nanomotors Advanced Design of Catalytic Nanomotors Applications, Challenges, and Perspectives RATIONAL DESIGN AND HIGH-THOUGHPUT SCREENING OF METAL OPEN FRAMEWORKS FOR GAS SEPARATION ND CATALYSIS Introduction MOF General Features and Brief State of the Art Combinatorial Design of MOF for CO2 Capture in a PSA Process MOF Design for Catalytic Application DESIGN OF BIMETALLIC CATALYSTS: FROM MODEL SURFACES TO SUPPORTED CATALYSTS Introduction Experimental and Theoretical Methods Results and Discussion SELF-ASSEMBLED MATERIALS FOR CATALYSIS Introduction Mesoscale Design Designing Catalysts at the Nanoparticle Surfaces THEORY-AIDED CATALYST DESIGN Introduction Catalytic Descriptors High-Throughput Simulation and Design Controlled-Patterning Catalyst Synthesis and Stability USE OF IN SITU XAS TECHNIQUES FOR CATALYSTS? CHARACTERIZATION AND DESIGN Introduction The X-Ray Absorption Techniques Recent Applications of X-Ray Absorption Techniques to the Design of Heterogeneous Catalysts Perspective CATALYST DESIGN THROUGH DUAL TEMPLATING Introduction Surfactant-Assisted Self-Assembly by Mesoporous Metal Oxides Colloidal Sphere Templating of Macroporous Metal Oxides Dual Templating of Metal Oxides Catalytic Applications

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